ONE-DIMENSIONAL MODEL FOR CALCULATING A NANOAEROSOL FLOW IN A CONTINUOUS REACTOR IN THE PRESENCE OF DIFFUSION AND COAGULATION OF PARTICLES

The infl uence of the deposition of nanoparticles of an aerosol, moving in a continuous reactor at a constant velocity, on the channel walls of the reactor and of the coagulation of these particles as a result of their Brownian diff usion on the nanoaerosol parameters was investigated. A simple one-dimensional model, adequately defi ning the diff usion, coagulation, and deposition of nanoaerosol particles in a wide range of change in its Knudsen number, has been constructed. It is shown analytically that, as the distance from the inlet of the reactor increases, the volume fraction of particles in the nanoaerosol decreases by the exponential law, and the radius of the clusters formed in the nanoaerosol as a result of the coagulation of its particles increases and tends to a limiting (maximum) value. A nonlinear integro-diff erential equation for the radius of such clusters has been obtained, and, from it, compact formulas for approximate calculation of its limiting radius have been derived. The characteristic distributions of the radii of clusters and of their concentrations along the reactor channel, calculated by the numerical method, are presented. It was established that, if this channel has a fairly large length, the clusters moving in it increase to their limiting size. The infl uence of the determining parameters of the fl ow of a nanoaerosol at the inlet to the continuous reactor on the distribution of its dispersion characteristics along the reactor channel, on the limiting size of the clysters in it, and on the characteristic length of the channel, at which the processes of deposition and coagulation of nanoaerosol particles are completed, is discussed. A comparison of the results of calculations of the parameters of a nanoaerosol moving in a continuous reactor by the one- and two-dimensional models has shown that the simple one-dimensional model defi nes the behavior of these parameters quite adequately.
The infl uence of the deposition of nanoparticles of an aerosol, moving in a continuous reactor at a constant velocity, on the channel walls of the reactor and of the coagulation of these particles as a result of their Brownian diff usion on the nanoaerosol parameters was investigated. A simple one-dimensional model, adequately defi ning the diff usion, coagulation, and deposition of nanoaerosol particles in a wide range of change in its Knudsen number, has been constructed. It is shown analytically that, as the distance from the inlet of the reactor increases, the volume fraction of particles in the nanoaerosol decreases by the exponential law, and the radius of the clusters formed in the nanoaerosol as a result of the coagulation of its particles increases and tends to a limiting (maximum) value. A nonlinear integro-diff erential equation for the radius of such clusters has been obtained, and, from it, compact formulas for approximate calculation of its limiting radius have been derived. The characteristic distributions of the radii of clusters and of their concentrations along the reactor channel, calculated by the numerical method, are presented. It was established that, if this channel has a fairly large length, the clusters moving in it increase to their limiting size. The infl uence of the determining parameters of the fl ow of a nanoaerosol at the inlet to the continuous reactor on the distribution of its dispersion characteristics along the reactor channel, on the limiting size of the clysters in it, and on the characteristic length of the channel, at which the processes of deposition and coagulation of nanoaerosol particles are completed, is discussed. A comparison of the results of calculations of the parameters of a nanoaerosol moving in a continuous reactor by the one- and two-dimensional models has shown that the simple one-dimensional model defi nes the behavior of these parameters quite adequately.
Author:  T. R. Amanbaev
Keywords:  nanoaerosol, continuous reactor, diff usion, deposition, coagulation, clusters, Knudsen number
Page:  1176